That would be a good idea. It's probably easiest to test the RAM first with
memtester. I can't remember whether it's a standard part of Raspbian Jessie or not, but you can soon install it with...
... if it's not there.
I believe you're running with GPU memory of 256MB, but you should still be able to test around 700MB of it without lowering that with...
...which will send it around one loop of extensive RAM tests. If it fails, knock the speed down a little. If it passes then run it at least another 5 times to be absolutely sure with...
That should keep you busy for the next few hours.
That CPU test is OK for starters, but a thorough workout of the CPUs and GPU together will be the ultimate test. That's why I mentioned Quake 3 Arena previously. It succeeds in crashing a borderline overclock where many stress tests fail.
